Photonic Multilayers for Broadband and Large Area Superchiral Surface Waves

Pellegrini G., Mogni E., Jil-Rostra J., Yubero F., Simone G., Fossati S., Dostálek J., Martinez Vázquez R., Osellame R., Celebrano M., Finazzi M., Biagioni P.

Chirality (in Nature)

Dipartimento di Fisica - Università di Pavia

ICTON2023, 2-6 July 2023, Bucharest, Romania

Molecules

DNA

Proteins

Left Enantiomer

Right Enantiomer

Probing Chirality with Electromagnetic Fields

Dipartimento di Fisica - Università di Pavia

ICTON2023, 2-6 July 2023, Bucharest, Romania

TM Polarization

Left = TE + i*TM

Right = TE - i*TM

Optical Rotation (OR)

Circular Dichroism (CD)

\[\mathrm{CD = A_{R}-A_{L}}\]

\[\mathrm{\psi = \Delta \theta} \]

TE Polarization

Superchiral Light: Enhancing Chiral Light-Matter Interaction

Dipartimento di Fisica - Università di Pavia

Finazzi, Marco, et al. "Quasistatic limit for plasmon-enhanced optical chirality." Physical Review B 91.19 (2015): 195427.

Schäferling, Martin. "Chiral nanophotonics." Springer Series in Optical Sciences 205 (2017): 159.

C = -\frac{\varepsilon_{0} \omega}{2} Im(\mathrm{\mathbf{E}}^{*} \cdot \mathrm{\mathbf{B}})

ICTON2023, 2-6 July 2023, Bucharest, Romania

Mattioli, F. et al. Plasmonic Superchiral Lattice Resonances in the Mid-Infrared. ACS Photonics 7, 2676–2681 (2020)

Superchiral Light with a Planar Geometry

Dipartimento di Fisica - Università di Pavia

  • Large optical chirality enhancement

  • Uniformity over large areas

  • Optical chirality switching

  • Broadband operation

  • Flat spectral response

Planar Geometries as an Ideal Candidate

ICTON2023, 2-6 July 2023, Bucharest, Romania

A Planar Geometry for Superchiral Light: Take 1

Dipartimento di Fisica - Università di Pavia

ICTON2023, 2-6 July 2023, Bucharest, Romania

TE ± i*TM

TE ± i*TM

Surface Plasmon

A Planar Geometry for Superchiral Light: Take 2

Dipartimento di Fisica - Università di Pavia

ICTON2023, 2-6 July 2023, Bucharest, Romania

Bloch Surface Waves (BSW)

TE ± i*TM

TE ± i*TM

\[ \mathrm{ (\lambda_{TM},\theta_{TM})} \]

\[ \mathrm{ (\lambda_{TE},\theta_{TE})} \]

\[ \mathrm{ (\lambda_{TM},\theta_{TM})} \neq \mathrm{ (\lambda_{TE},\theta_{TE})} \]

Superchiral Surface Waves with SiO2-Ta2O5 1PDC

Dipartimento di Fisica - Università di Pavia

  • Pellegrini, Giovanni, et al. "Chiral surface waves for enhanced circular dichroism." Physical Review B 95.24 (2017): 241402.

  • Pellegrini, Giovanni, et al. "Surface‐enhanced chiroptical spectroscopy with superchiral surface waves." Chirality 30.7 (2018): 883-889.

  • Pellegrini, Giovanni, et al. "Superchiral surface waves for all-optical enantiomer separation." The Journal of Physical Chemistry C 123.46 (2019): 28336-28342.

ICTON2023, 2-6 July 2023, Bucharest, Romania

Towards Surface Mode Polarization Control

Dipartimento di Fisica - Università di Pavia

Mogni, Erika, et al. "One‐Dimensional Photonic Crystal for Surface Mode Polarization Control." Advanced Optical Materials (2022): 2200759.

ICTON2023, 2-6 July 2023, Bucharest, Romania

Genetically Evolved Superchiral Photonics Crystals

Dipartimento di Fisica - Università di Pavia

ICTON2023, 2-6 July 2023, Bucharest, Romania

SiO\(_{2}\)

Ta\(_{2}\)O\(_{5}\)

Genetically Evolved Organic Superchiral Photonics Crystals

Dipartimento di Fisica - Università di Pavia

Polystyrene

Cellulose

ICTON2023, 2-6 July 2023, Bucharest, Romania

Pellegrini G., Mogni E., Jil-Rostra J., Yubero F., Simone G., Fossati S., Dostálek J., Martinez Vázquez R., Osellame R., Celebrano M., Finazzi M., Biagioni P.

SuperchiralSpectroscopy

By Giovanni Pellegrini

SuperchiralSpectroscopy

  • 50