Spiral - Modeling of Superchiral Surface Waves

Chirality (in Nature)

Dipartimento di Fisica - Università di Pavia

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Molecules

DNA

Proteins

Left Enantiomer

Right Enantiomer

Probing Chirality with Electromagnetic Fields

Dipartimento di Fisica - Università di Pavia

TM Polarization

Left = TE + i*TM

Right = TE - i*TM

Optical Rotation (OR)

Circular Dichroism (CD)

\[\mathrm{CD = A_{R}-A_{L}}\]

\[\mathrm{\psi = \Delta \theta} \]

TE Polarization

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Superchiral Light: Enhancing Chiral Light-Matter Interaction

Dipartimento di Fisica - Università di Pavia

Finazzi, Marco, et al. "Quasistatic limit for plasmon-enhanced optical chirality." Physical Review B 91.19 (2015): 195427.

Schäferling, Martin. "Chiral nanophotonics." Springer Series in Optical Sciences 205 (2017): 159.

C = -\frac{\varepsilon_{0} \omega}{2} Im(\mathrm{\mathbf{E}}^{*} \cdot \mathrm{\mathbf{B}})

Mattioli, F. et al. Plasmonic Superchiral Lattice Resonances in the Mid-Infrared. ACS Photonics 7, 2676–2681 (2020)

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Superchiral Light with a Planar Geometry

Dipartimento di Fisica - Università di Pavia

  • Large optical chirality enhancement

  • Uniformity over large areas

  • Optical chirality switching

  • Broadband operation

  • Flat spectral response

Planar Geometries as an Ideal Candidate

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

A Planar Geometry for Superchiral Light: Take 1

Dipartimento di Fisica - Università di Pavia

TE ± i*TM

TE ± i*TM

Surface Plasmon

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

A Planar Geometry for Superchiral Light: Take 2

Dipartimento di Fisica - Università di Pavia

Bloch Surface Waves (BSW)

TE ± i*TM

TE ± i*TM

\[ \mathrm{ (\lambda_{TM},\theta_{TM})} \]

\[ \mathrm{ (\lambda_{TE},\theta_{TE})} \]

\[ \mathrm{ (\lambda_{TM},\theta_{TM})} \neq \mathrm{ (\lambda_{TE},\theta_{TE})} \]

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Superchiral Surface Waves with SiO2-Ta2O5 1PDC

Dipartimento di Fisica - Università di Pavia

  • Pellegrini, Giovanni, et al. "Chiral surface waves for enhanced circular dichroism." Physical Review B 95.24 (2017): 241402.

  • Pellegrini, Giovanni, et al. "Surface‐enhanced chiroptical spectroscopy with superchiral surface waves." Chirality 30.7 (2018): 883-889.

  • Pellegrini, Giovanni, et al. "Superchiral surface waves for all-optical enantiomer separation." The Journal of Physical Chemistry C 123.46 (2019): 28336-28342.

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Towards Surface Mode Polarization Control

Dipartimento di Fisica - Università di Pavia

Mogni, Erika, et al. "One‐Dimensional Photonic Crystal for Surface Mode Polarization Control." Advanced Optical Materials (2022): 2200759.

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Genetically Evolved Superchiral Photonics Crystals

Dipartimento di Fisica - Università di Pavia

SiO\(_{2}\)

Ta\(_{2}\)O\(_{5}\)

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Genetically Evolved Organic Superchiral Photonics Crystals

Dipartimento di Fisica - Università di Pavia

Polystyrene

Cellulose

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Operating in "Optical Rotation" Mode

Dipartimento di Fisica - Università di Pavia

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Three Materials Design: Fighting the Brewster Angle

Dipartimento di Fisica - Università di Pavia

Spiral Kickoff Meeting, 3 October 2023, Polimi, Milano

Spiral - Unipv

By Giovanni Pellegrini

Spiral - Unipv

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